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Given the photocatalytic properties of semiconducting polymers and carbon quantum dots (CQDs), we report a new structure for a metal-free photocatalytic system with a promising efficiency for hydrogen production through the combination of an organic semiconducting polymer (PFTBTA) and N-doped carbon quantum dots (NCQDs) covered by PS-PEGCOOH to produce heterostructured photocatalysts in the form o

In this communication, we present the phase diagram of CsPb(BrxI1-x)3 (0 ≤ x ≤ 1, 300-585 K) obtained by high-throughput in situ GIWAXS measurements of a combinatorial thin film library. We find that all compositions convert to the cubic perovskite phase at high temperature and that the presence of bromide in the films stabilizes the metastable perovskite phases upon cool down. In accordance with

Background and purpose — Obesity is a considerable medical challenge in society. We investigated the risk of revision for any reasons and for infection in patients having total knee arthroplasty (TKA) for osteoarthritis (OA) within 2 years after bariatric surgery (BS) and compared them with TKAs without BS. Patients and methods — We used the Scandinavian Obesity Surgery Registry (SOReg) and the Sw

We prepared triplet-triplet annihilation photon upconverters combining thin-film methylammonium lead iodide (MAPI) perovskite with a rubrene annihilator in a bilayer structure. Excitation of the perovskite film leads to delayed, upconverted photoluminescence emitted from the annihilator layer, with triplet excitation of the rubrene being driven by carriers excited in the perovskite layer. To bette

Recently, intense research activities have been focused on solution-processed hybrid lead halide perovskite semiconductors which are being developed for the solar-cell, light emitting diode (LED), and lasing applications. To optimize and fabricate a competitive perovskite-based optoelectronic device, the fundamental studies of the electronic structure, photo-generated carrier dynamics as well as t

A new modification of a table-Top laser-driven water-jet plasma X-ray source has been successfully implemented and commissioned at the Extreme Light Infrastructure (ELI) Beamlines user facility. In order to preserve the broadband nature of the source for spectroscopic experiments, a polycapillary lens was initially chosen as the focusing element. Generally, polycapillary X-ray optics have a narrow

Plasmon hot carriers are interesting for photoredox chemical synthesis but their direct utilization is limited by their ultrafast thermalization. Therefore, they are often transferred to suitable accepting materials that expedite their lifetime. Solid-state photocatalysts are technologically more suitable than their molecular counterparts, but their photophysical processes are harder to follow due

Rationale: Symptom relief is a key treatment goal in patients with chronic obstructive pulmonary disease (COPD). However, there are limited data available on the response to bronchodilator therapy in patients at low risk of exacerbations with different levels of symptom severity. This study compared treatment responses in patients with a range of symptom severities as indicated by baseline COPD as

Background and purpose — The population of the Nordic countries is aging and the number of elderly patients undergoing total knee arthroplasty (TKA) is also expected to increase. Reliable fixation methods are essential to avoid revisions. We compared the survival of different TKA fixation concepts with cemented fixation as the gold standard. Patients and methods — We used data from the Nordic Arth

The spin polarization in centrosymmetric molybdenum disulfide (MoS2) bulk crystal is recorded by helicity dependent photocurrent exposed as elliptically polarized terahertz (THz) emission. We assign this observation to hidden spin polarization due to the local Dresselhaus effect induced by the molybdenum atomic site asymmetry. This spin polarization induces ultrafast optically controlled circular

Long charge carrier diffusion length and large grain size are commonly believed to be inherent properties of highly luminescent polycrystalline thin-film semiconductors. However, exactly these two properties make luminescence very susceptible to quenching by just one strongly quenching defect state if present in each grain. Moreover, when the number of quenchers per grain is small (say 1–10), it v

Attosecond pulses, produced through high-order harmonic generation in gases, have been successfully used for observing ultrafast, subfemtosecond electron dynamics in atoms, molecules and solid state systems. Today's typical attosecond sources, however, are often impaired by their low repetition rate and the resulting insufficient statistics, especially when the number of detectable events per shot

The research about how a nanoparticle (NP) interacts with a complex biological solution has been conducted, according to the literature, for almost three decades. A significant amount of data has been generated, especially in the last one and a half decade. First, it became its own research field which was later divided into many subresearch fields. This outlook does not aim to be a comprehensive

Finite fermion systems are known to exhibit shell structure in the weakly interacting regime, as is well known from atoms, nuclei, metallic clusters, or even quantum dots in two dimensions. All these systems have in common that the particle interactions between electrons or nucleons are spatially isotropic. Dipolar quantum systems as they have been realized with ultracold gases, however, are gover

Precise thermometry is of wide importance in science and technology in general and in quantum systems in particular. Here, we investigate fundamental precision limits for thermometry on cold quantum systems, taking into account constraints due to finite measurement resolution. We derive a tight bound on the optimal precision scaling with temperature, as the temperature approaches zero. The bound d

Adiabatic elimination methods allow the reduction of the space dimension needed to describe systems whose dynamics exhibit separation of timescale. For open quantum systems, it consists in eliminating the fast part assuming it has almost instantaneously reached its steady state and obtaining an approximation of the evolution of the slow part. These methods can be applied to eliminate a linear subs

Vacancy-ordered lead-free perovskites with more-stable crystalline structures have been intensively explored as the alternatives for resolving the toxic and long-term stability issues of lead halide perovskites (LHPs). The dispersive energy bands produced by the closely packed halide octahedral sublattice in these perovskites are meanwhile anticipated to facility the mobility of charge carriers. H